In the app (the quickest): Settings → Account → Delete account. Confirm with your password, or by picking your Google account again. The account is gone at once.
Write to gamedev@ittt-production.uk from the email address of your account, with the subject Delete my account. I'll confirm and delete it within 30 days, usually much sooner. If you signed in with Google, write from that Google account's address.
More in the privacy policy.